Fischer–Tropsch conversion of biomass‐derived synthesis gas to liquid fuels
Identifieur interne : 000309 ( Main/Exploration ); précédent : 000308; suivant : 000310Fischer–Tropsch conversion of biomass‐derived synthesis gas to liquid fuels
Auteurs : Andreas Helland Lilleb [Norvège] ; Anders Holmen [Norvège] ; Bj Rn Christian Enger [Norvège] ; Edd Anders Blekkan [Norvège]Source :
- Wiley Interdisciplinary Reviews: Energy and Environment [ 2041-8396 ] ; 2013-09.
Abstract
Recent and ongoing research on Fischer–Tropsch catalysts for biomass conversion typically focus on the effects of impurities common in bio‐derived synthesis gas, and also on the effect of different synthesis gas compositions expected from biomass gasifiers. Cobalt and iron catalysts share the sensitivity toward some, but not all of the impurities. The most profound difference is the strong negative effect of alkali, alkaline earth, and nitrogen containing compounds on cobalt catalysts while these impurities have a negligible or no effect on iron catalysts. CO2 appears to mainly act as a diluent in cobalt‐based processes while iron catalysts respond differently to this component depending on catalyst design. In particular, iron catalysts containing Al2O3 as a structural promoter display a high stability, C5+ selectivity, and activity in CO2 rich synthesis gas.
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DOI: 10.1002/wene.69
Affiliations:
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Interdisciplinary Reviews: Energy and Environment</title><title level="j" type="abbrev">WENE</title><idno type="ISSN">2041-8396</idno><idno type="eISSN">2041-840X</idno><imprint><publisher>Blackwell Publishing Ltd</publisher><date type="published" when="2013-09">2013-09</date><biblScope unit="volume">2</biblScope><biblScope unit="issue">5</biblScope><biblScope unit="page" from="507">507</biblScope><biblScope unit="page" to="524">524</biblScope></imprint><idno type="ISSN">2041-8396</idno></series><idno type="istex">A6361073D7682ACF5537ED961B405437CB0AEB4C</idno><idno type="DOI">10.1002/wene.69</idno><idno type="ArticleID">WENE69</idno></biblStruct></sourceDesc><seriesStmt><idno type="ISSN">2041-8396</idno></seriesStmt></fileDesc><profileDesc><textClass></textClass><langUsage><language ident="en">en</language></langUsage></profileDesc></teiHeader><front><div type="abstract">Recent and ongoing research on Fischer–Tropsch catalysts for biomass conversion typically focus on the effects of impurities common in bio‐derived synthesis gas, and also on the effect of different synthesis gas compositions expected from biomass gasifiers. Cobalt and iron catalysts share the sensitivity toward some, but not all of the impurities. The most profound difference is the strong negative effect of alkali, alkaline earth, and nitrogen containing compounds on cobalt catalysts while these impurities have a negligible or no effect on iron catalysts. CO2 appears to mainly act as a diluent in cobalt‐based processes while iron catalysts respond differently to this component depending on catalyst design. In particular, iron catalysts containing Al2O3 as a structural promoter display a high stability, C5+ selectivity, and activity in CO2 rich synthesis gas.</div></front></TEI><affiliations><list><country><li>Norvège</li></country><region><li>Trøndelag</li></region><settlement><li>Trondheim</li></settlement></list><tree><country name="Norvège"><region name="Trøndelag"><name sortKey="Lilleb, Andreas Helland" sort="Lilleb, Andreas Helland" uniqKey="Lilleb A" first="Andreas Helland" last="Lilleb">Andreas Helland Lilleb</name></region><name sortKey="Blekkan, Edd Anders" sort="Blekkan, Edd Anders" uniqKey="Blekkan E" first="Edd Anders" last="Blekkan">Edd Anders Blekkan</name><name sortKey="Enger, Bj Rn Christian" sort="Enger, Bj Rn Christian" uniqKey="Enger B" first="Bj Rn Christian" last="Enger">Bj Rn Christian Enger</name><name sortKey="Holmen, Anders" sort="Holmen, Anders" uniqKey="Holmen A" first="Anders" last="Holmen">Anders Holmen</name></country></tree></affiliations></record>Pour manipuler ce document sous Unix (Dilib)
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